Poster Presentation 11th Australian Peptide Conference 2015

Techniques to study cholesterol dependent citolysins (CDCs) binding  to cholesterol containing membranes (#141)

Mirijam Kozorog 1 2 , Marc-Antoine Sani 2 , Frances Separovic 2 , Gregor Anderluh 1 3
  1. National Institute of Chemistry, Ljubljana, Slovenia
  2. School of Chemistry/Bio21 Institute, The Univerity of Melbourne, Melbourne, VIC
  3. Department of Biology, University of Ljubljana, Biotechnical Faculty, Ljubljan, Slovenia
Cholesterol dependent citolysins (CDCs)  are a family of pore-forming proteins, expressed by various bacterial species. They are all secreted as soluble monomers that bind to membrane cholesterol, oligomerise and form pores up to 35 nm in diameter. Pore formation triggers also numerous other cellular effects, such us endocytosis, histone modification, activation of kinases and others. Lately our study have been focused on listeriolysin O, a pH dependent CDC that is expressed by human pathogen G+ bacteria Listeria monocytogenes. The bacteria causes listeriosis, which starts with the ingestion of contaminated foods and affects mainly immunocompromised persons and pregnant women. Infection during pregnancy can result in life-threatening infection of the newborns, and also 30 % of infections in adults result in death. Besides being the main viruence factor of Listeria, is LLO interesting also for its pH dependent pore-forming activity which has a potential to be used for targeted drug delivery system in a combination with suitable membrane sistem therefore the understanding of its membrane binding events is crucial for further experiment design. For LLO's membrane binding study several artificial membrane systems with high cholesterol level were prepared (large, small and giant multilamellar vesicles, and nanodiscs) with different lipid composition. Calcein release, centrifugation assay, hemolysis, SPR and NMR experiments were performed to gain more insight into binding at molecular level. LLO was also labelled with Alexa Fluor A488 and its binding to artificial membrane vesicles was observed with confocal microscopy. We confirmed LLO's specific cholesterol-dependent binding and introduced new techniques in lipid vesicles preparation, such as nanodiscs, composed of archaeal lipids w/o cholesterol, which are of special interest since arcaeal lipids are known to be among most stable one.